TY - JOUR
T1 - Dynamical thermoelectric transport properties of graphene
T2 - MF approach
AU - Rani, Luxmi
AU - Han, Jeong In
N1 - Publisher Copyright:
© 2023 Elsevier Ltd
PY - 2023/11
Y1 - 2023/11
N2 - In the present work, Seebeck coefficient and Figure of merit in terms of thermoelectric, electric, and thermal scattering rates employing powerful technique of memory function formalism in graphene system are investigated. This study leads to the dynamical thermoelectric transport behavior of graphene subjected to electron–phonon interactions using linear response theory. Within premises, explicit expression of generalized Drude scattering rate or imaginary part of memory function associated with thermoelectric/electric/thermal functions is studied. In zero frequency (DC regime) and low-temperature limit, Seebeck coefficient shows the linear-T dependence and, is found to be good in agreement with the experimental and theoretical results. Further, several frequency and temperature dependent transport coefficient results for electron–phonon scattering in graphene are performed. We found that S(ω,T) shows saturation at ω≫ωBG and raises with temperature below the Bloch–Grüneisen (BG) frequency regime (ω≪ωBG). We numerically investigated thermoelectric Figure of merit (ZT) with frequency/temperature domains and discussed.
AB - In the present work, Seebeck coefficient and Figure of merit in terms of thermoelectric, electric, and thermal scattering rates employing powerful technique of memory function formalism in graphene system are investigated. This study leads to the dynamical thermoelectric transport behavior of graphene subjected to electron–phonon interactions using linear response theory. Within premises, explicit expression of generalized Drude scattering rate or imaginary part of memory function associated with thermoelectric/electric/thermal functions is studied. In zero frequency (DC regime) and low-temperature limit, Seebeck coefficient shows the linear-T dependence and, is found to be good in agreement with the experimental and theoretical results. Further, several frequency and temperature dependent transport coefficient results for electron–phonon scattering in graphene are performed. We found that S(ω,T) shows saturation at ω≫ωBG and raises with temperature below the Bloch–Grüneisen (BG) frequency regime (ω≪ωBG). We numerically investigated thermoelectric Figure of merit (ZT) with frequency/temperature domains and discussed.
KW - Graphene
KW - Memory function formalism
KW - Seebeck coefficient
KW - Thermoelectric figure of merit
KW - Thermoelectronic transport in graphene
UR - http://www.scopus.com/inward/record.url?scp=85167805818&partnerID=8YFLogxK
U2 - 10.1016/j.jpcs.2023.111583
DO - 10.1016/j.jpcs.2023.111583
M3 - Article
AN - SCOPUS:85167805818
SN - 0022-3697
VL - 182
JO - Journal of Physics and Chemistry of Solids
JF - Journal of Physics and Chemistry of Solids
M1 - 111583
ER -