Solid electrolyte-electrode interface based on buffer therapy in solid-state lithium batteries

Lei ying Wang, Li fan Wang, Rui Wang, Rui Xu, Chun Zhan, Woochul Yang, Gui cheng Liu

Research output: Contribution to journalReview articlepeer-review

14 Scopus citations

Abstract

In the past few years, the all-solid lithium battery has attracted worldwide attentions, the ionic conductivity of some all-solid lithium-ion batteries has reached 10−3–10−2 S/cm, indicating that the transport of lithium ions in solid electrolytes is no longer a major problem. However, some interface issues become research hotspots. Examples of these interfacial issues include the electrochemical decomposition reaction at the electrode-electrolyte interface; the low effective contact area between the solid electrolyte and the electrode etc. In order to solve the issues, researchers have pursued many different approaches. The addition of a buffer layer between the electrode and the solid electrolyte has been at the center of this endeavor. In this review paper, we provide a systematic summarization of the problems on the electrode-solid electrolyte interface and detailed reflection on the latest works of buffer-based therapies, and the review will end with a personal perspective on the improvement of buffer-based therapies.

Original languageEnglish
Pages (from-to)1584-1602
Number of pages19
JournalInternational Journal of Minerals, Metallurgy and Materials
Volume28
Issue number10
DOIs
StatePublished - Oct 2021

Keywords

  • buffer layer
  • interface
  • solid electrolyte
  • solid-state lithium-ion batteries

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